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When using the Item (get_Item) property of the ExToolBar.CRD/COM component on VB.NET environment, in VB/NET, it throws a compiler error:

error BC30456: 'get_Item' is not a member of 'AxEXTOOLBARCRDLib.AxToolBarCRD'

so, instead using the get_Item, you have to use the Item accessor instead as in the following sample.

The correct syntax would be:

With .Item(100)
    .Caption = "Just a caption"
End With

instead of:

With .get_Item(100)
    .Caption = "Just a caption"
End With